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Experimental ARPES resolution

The ARPES experimental resolution depends on several factors including measurement temperature, sample quality, quality of electrical contact between sample and analyzer, light source used, and the analyzer resolution. Here we will describe a practical scenario. The sample for this measurement was grown using molecular beam epitaxy (MBE) method. The sample was of very good quality. We obtained the following ARPES spectrum using 10 eV pass energy and 5 meV energy step.

res-band

We extract the Energy Distribution Curve (EDC) by integrating ±0.25 Å-1 range.

res-edc

Thermal broadening is given by Fermi Dirac distribution:

F(ϵ)=1e(ϵμ)/kBT+1F(\epsilon) = \frac{1}{e^{(\epsilon - \mu)/k_B T} + 1}

Above measurement was carried out at liquid nitrogen temperature; the sample temperature reaches about 90 K, at which the Fermi-Dirac distribution looks like this:

res-fermi-func

Now, we can convolute a Gaussian broadening of 10 meV, which fits our experimental data well.

res-fit

There is some room for adjusting the fitting parameters, but the slope is certainly better than 15 meV for our current data. Therefore, we have about 8 meV thermal broadening at 90 K and 10 meV instrumental (combines analyzer resolution, light source broadening etc.), i.e., we can expect better than 15 meV (σtotalσx2+σy2)(\sigma_{total} \le \sqrt{\sigma_x^2 + \sigma_y^2}) resolution.